Abstract
Fine particles (PM2.5) are harmful to human health especially during periods of limited dispersion when the concentrations build up. This is a common occurrence in Southern Brazil in the dry season when high-pressure stationary systems inhibit vertical dispersion and reduce wind speed. The objective of this study was to evaluate the PM2.5 concentrations in the Region of Greater Vitória during the winter of 2013, and to assess the influence of the large-scale meteorological circulation on its concentration. An experimental campaign was carried out to determine the mass of PM2.5 at six urban sites and particle number concentration. The average PM2.5 concentrations varied from 9.70 μg m-3 to 14.36 μg m-3 with the average daily maximum reaching 29.35 μg m-3, exceeding the World Health Organization guideline (24-h average: 25 μg m-3). The particle size distribution showed a larger number of particles from 18 to 21 h (local time), indicating that the main vehicular emissions are the main sources. During the winter, rainfall associated with cold fronts were responsible for a decrease in the particulate concentrations. In contrast, the occurrence of high-pressure systems led to an increase in particle concentrations, due to stagnant conditions.
Keywords:
fine particles; meteorological parameters; urban area; particle counting; particle size distribution; winter
