Recent advances in layered double hydroxides applied to photoprotection

Silva, Tamires Andrade da; Silva, Tamares Andrade da; Nascimento, Ticiano Gomes do; Yatsuzuka, Rebeca Evahides; Grillo, Luciano Aparecido Meireles; Dornelas, Camila Braga

doi:10.31744/einstein_journal/2019RW4456

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REVIEW • Einstein (São Paulo) 17 (1) • 2019 • https://doi.org/10.31744/einstein_journal/2019RW4456 copy

Recent advances in layered double hydroxides applied to photoprotection

Authorship SCIMAGO INSTITUTIONS RANKINGS

ABSTRACT

Layered double hydroxides have received more attention from researchers due to their range of applications, ease of synthesis and low cost of production. With broader knowledge about solar radiation effects on the body, the use of sunscreens has become even more important. The ability of some nanostructures, such as layered double hydroxides, to act as matrices has made it possible to obtain improvements in photoprotective formulations, with solutions to problems caused by radiation and sunscreens. This review article brings together the most recent advances of these clays, the layered double hydroxides, applied to photoprotection.

Nanotechnology; Nanostructures; Clay; Solar radiation; Ultraviolet filters

Authors	LDH	UV absorber	Method
Khan et al.⁽¹1. Khan SB, Liu C, Jang ES, Akhtar K, Han H. Encapsulation of organic UV ray absorbents into layered double hydroxide for photochemical properties. Mater Lett. 2011;65(19-20):2923-6.⁾	ZnAl	3,4-dihydroxycinnamic acid (cinnamic acid)	Co-precipitation
		4-hydroxy-3,5-dimethoxycinnamic acid (SA)
		3-amino-5-trifluoromethylbenzoic acid (FBA)
Li et al.⁽²2. Li S, Shen Y, Xiao M, Liu D, Fa L, Wu K. Intercalation of 2,4-dihydroxybenzophenone-5-sulfonate anion into Zn/Al layered double hydroxides for UV absorption properties. Ind Eng Chem. 2014;20(4):1280-4.⁾	ZnAl	2,4-dihydroxybenzophenone-5-sulfonate	Co-precipitation
Li et al.⁽²⁴24. Li Y, Tang L, Ma X, Wang X, Zhou W, Bai D. Synthesis and characterization of Zn-Ti layered double hydroxide intercalated with cinnamic acid for cosmetic application. J Phys Chem Solids. 2017;107:62-7.⁾	ZnTi	Cinnamic acid	Ion-exchange
Wang et al.⁽²⁵25. Wang XR, Li Y, Tang LP, Gan W, Zhou W, Zhao YF, et al. Fabrication of Zn-Ti layered double hydroxide by varying cationic ratio of Ti4+ and its application as UV absorbent. Chin Chem Lett. 2017;28(2):394-9.⁾	MgAl	Zinc	Co-precipitation
	ZnAl	Titanium salts
	ZnTi
He et al.⁽²⁶26. He Q, Yin S, Sato T. Synthesis and photochemical properties of zinc–aluminum layered double hydroxide/organic UV ray absorbing molecule/silica nanocomposites. J Phys Chem Solids. 2004;65(2-3):395-402.⁾	ZnAl	4-hydroxy-3-methoxybenzoic acid	Anion-exchange and/or co-precipitation
		2-hydroxy-4-methoxybenzophenone-5-sulfonic acid
		4-hydroxy-3-methoxycinnamic acid
		4,4’-diaminostilbene-2,2’-disulfonic acid
		p-aminobenzoic acid
		Urocanic acid
Sun et al.⁽²⁷27. Sun W, He Q, Lu L, Liu H. Synthesis and properties of layered double hydroxides intercalated with cinnamic acid series organic UV ray absorbents. Mater Chem Phys. 2008;107(2-3):261-5.⁾	ZnAl	Cinnamic acid	Co-precipitation
		3,4-dimethoxycinnamic acid
		p-hydroxycinnamic acid
Li et al.⁽²⁸28. Li Y, Tang LP, Zhou W, Wang XR. Fabrication of intercalated p-aminobenzoic acid into Zn-Ti layered double hydroxide and its application as UV absorbent. Chin Chem Lett. 2016;27(9):1495-9.⁾	ZnTi	p-aminobenzoic acid	Ion-exchange
Sun et al.⁽²⁹29. Sun W, He Q, Luo Y. Synthesis and properties of cinnamic acid series organic UV ray absorbents–interleaved layered double hydroxide. Mater Lett. 2007;61(8-9):1881-4.⁾	ZnAl	Cinnamic acid	Co-precipitation
		p-methoxycinnamic acid
Perioli et al.⁽³⁰30. Perioli L, Ambrogi V, Bertini B, Ricci M, Nocchetti M, Latterini L, et al. Anionic clays for sunscreen agent safe use: photoprotection, photostability and prevention of their skin penetration. Eur J Pharm Biopharm. 2006;62(2):185-93.⁾	MgAl	p-aminobenzoic acid	Anion-exchange
	ZnAl
Perioli et al.⁽³¹31. Perioli L, Ambrogi V, Rossi C, Latterini L, Nocchetti M, Costantino U. Use of anionic clays for photoprotection and sunscreen photostability: hydrotalcites and phenylbenzimidazole sulfonic acid. J Phys Chem Solids. 2006;67(5-6):1079-83.⁾	MgAl	2-phenyl-1H-benzimidazole-5-sulfonic acid (Eusolex 232)	Anion-exchange and/or co-precipitation reaction
	ZnAl
Perioli et al.⁽³²32. Perioli L, Nocchetti M, Ambrogi V, Latterini L, Rossi C, Costantino U. Sunscreen immobilization on ZnAl-hydrotalcite for new cosmetic formulations. Microporous Mesoporous Mater. 2008;107(1-2):180-9.⁾	ZnAl	5-benzoyl-4-hydroxy-2-methoxy-benzenesulphonate acid	Ion-exchange
Cursino et al.⁽³³33. Cursino AC, Lisboa FS, Pyrrho AS, de Sousa VP, Wypych F. Layered double hydroxides intercalated with anionic surfactants/benzophenone as potential materials for sunscreens. J Colloid Interface Sci. 2013;397:88-95.⁾	ZnAl	Dodecylsulfate	Co-precipitation
		Dodecylbenzenesulfonate
Mohsin et al.⁽³⁴34. Mohsin SM, Hussein MZ, Sarijo SH, Fakurazi S, Arulselvan P, Taufiq-Yap YH. Optimization of UV absorptivity of layered double hydroxide by intercalating organic UV-absorbent molecules. J Biomed Nanotechnol. 2014;10(8):1490-500.⁾	ZnAl	Benzophenone 9	Co-precipitation and ion exchange

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[1] Corresponding author: Camila Braga Dornelas. Campus A. C. Simões. Avenida Lourival Melo Mota, s/n. Tabuleiro do Martins. Zip code: 57072-900 – Maceió, AL, Brazil. Phone: (55 82) 3214-1154. E-mail: dornelascb@yahoo.com.br